Move to frame 29 (he's saying "Ludwig") and rotate his head down a bit. Insert its location and rotation.
Move to frame 36 (because why not?) and rotate his head back up. Insert it's location and rotation.
Now move to frame 46, and rotate the head up juuuuuuuuust a tiiiiiiny bit. You're never entirely still, you know.
Now move to frame 53 and rotate his head back and to the left.
Now back to frame 46 and insert the location of the EyeTarget.
Frame 50 (3 frames before his head finishes moving) move the eyes up and to the right.
Frame 63, rotate the head back and to the right juuuuuuust a tiiiiiiny bit.
Frame 69, rotate the head clockwise (from topview) and tilt it to the left a bit.
Frame 63, insert the location of the EyeTarget.
Frame 66 (before the head finishes moving again) move the eyes to the left.